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Titanium(IV) nitrate

Titanium nitrate is the inorganic compound with formula Ti(NO<sub>3</sub>)<sub>4</sub>. It is a colorless, diamagnetic solid that sublimes readily. It is an unusual example of a volatile binary transition metal nitrate. Ill defined species called titanium nitrate are produced upon dissolution of titanium or its oxides in nitric acid.

Preparation

Similarly to its original method, Ti(NO<sub>3</sub>)<sub>4</sub> is prepared by the nitration of titanium tetrachloride using dinitrogen pentoxide or chlorine nitrate:

TiCl<sub>4</sub> + 4 N<sub>2</sub>O<sub>5</sub> → Ti(NO<sub>3</sub>)<sub>4</sub> + 4 ClNO<sub>2</sub>

Hydrated titanium nitrate, the nitrate salt of the aquo complex [Ti(H<sub>2</sub>O)<sub>6</sub>]<sup>3+</sup>, is produced upon dissolution of titanium compounds in nitric acid.

Structure

The complex has D<sub>2d</sub> symmetry, with four bidentate nitrate ligands. The N-O distances are 1·29&nbsp;Å and 1·185&nbsp;Å (noncoordinated).

Physical properties

In the infrared spectrum, it absorbs strongly at 1635&nbsp;cm<sup>−1</sup>, assigned to a N-O vibrational mode.

It is soluble in nonpolar solvents silicon tetrachloride and carbon tetrachloride.

Reactions

Titanium nitrate is hygroscopic, converting to ill-defined hydrates. The anhydrous material is highly reactive, even toward hydrocarbons. Titanium nitrate also reacts with n-dodecane, p-dichlorobenzene, anisole, and biphenyl.

It decomposes thermally to titanium dioxide.

References

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