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Tetrabenzylzirconium

Tetrabenzylzirconium is an organozirconium compound with the formula Zr(CH<sub>2</sub>C<sub>6</sub>H<sub>5</sub>)<sub>4</sub>. The molecule features diamagnetic Zr(IV) bonded to four benzyl ligands. It is an orange air- and photo-sensitive solid, which is soluble in hydrocarbon solvents. The compound is a precursor to catalysts for the polymerization of olefins.

Structure, synthesis, reactions

X-ray crystallography demonstrates that the benzyl ligands are highly flexible: one polymorph features four η<sup>2</sup>-ligands, whereas another has two η<sup>1</sup>- and two η<sup>2</sup>-benzyl ligands.

The compound is prepared by combining benzylmagnesium chloride and zirconium tetrachloride in diethyl ether.

Tetrabenzylzirconium readily undergoes protonolysis, e.g. with hydrogen chloride:

Zr(CH<sub>2</sub>C<sub>6</sub>H<sub>5</sub>)<sub>4</sub> + HCl → Zr(CH<sub>2</sub>C<sub>6</sub>H<sub>5</sub>)<sub>3</sub>Cl + CH<sub>3</sub>C<sub>6</sub>H<sub>5</sub>

References