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Peroxynitrite

Peroxynitrite (sometimes called peroxonitrite) is an ion with the formula ONOO<sup>−</sup>. It is a structural isomer of nitrate, . Peroxynitrite is a potent reactive nitrogen species and is highly cytotoxic.

Preparation

Peroxynitrite can be prepared by the reaction of superoxide with nitric oxide:

It is prepared by the reaction of hydrogen peroxide with nitrite:

H<sub>2</sub>O<sub>2</sub> + → ONOO<sup>−</sup> + H<sub>2</sub>O

Its presence is indicated by the absorbance at 302&nbsp;nm (pH&nbsp;12, ε<sub>302</sub>&nbsp;=&nbsp;1670&nbsp;M<sup>−1</sup>&nbsp;cm<sup>−1</sup>).

Reactions

Peroxynitrite is weakly basic with a pK<sub>a</sub> of ~6.8.

It is reactive toward DNA and proteins.

ONOO<sup>−</sup> reacts nucleophilically with carbon dioxide. In vivo, the concentration of carbon dioxide is about 1 mM, and its reaction with ONOO<sup>−</sup> occurs quickly. Thus, under physiological conditions, the reaction of ONOO<sup>−</sup> with carbon dioxide to form nitrosoperoxycarbonate () is by far the predominant pathway for ONOO<sup>−</sup>. homolyzes to form carbonate radical and nitrogen dioxide, again as a pair of caged radicals. Approximately 66% of the time, these two radicals recombine to form carbon dioxide and nitrate. The other 33% of the time, these two radicals escape the solvent cage and become free radicals. It is these radicals (carbonate radical and nitrogen dioxide) that are believed to cause peroxynitrite-related cellular damage.

Peroxynitrous acid

Its conjugate acid peroxynitrous acid is highly reactive, although peroxynitrite is stable in basic solutions.

See also

References