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Diboron tetrachloride

Diboron tetrachloride is a tetrahalodiborane chemical compound with the formula B<sub>2</sub>Cl<sub>4</sub>. It is a colorless liquid.

Synthesis

The modern synthesis involves the chlorination of diboron tetrabromide by gallium(III) chloride.

It can also be formed by the electrical discharge procedure of boron trichloride at low temperatures:

BCl<sub>3</sub> → BCl<sub>2</sub> + Cl
Cl + Hg (electrode) → Hg<sub>2</sub>Cl<sub>2</sub> or HgCl<sub>2</sub>
2 BCl<sub>2</sub> → B<sub>2</sub>Cl<sub>4</sub>

The most efficient synthesis technique uses no dechlorinating metal, instead passing radio-frequency alternating current through gaseous boron trichloride.

Structure

The molecular structure of diboron tetrachloride, B<sub>2</sub>Cl<sub>4</sub>, was determined by gas electron diffraction. The molecules have D<sub>2d</sub> symmetry, i.e. the two planar BBCl<sub>2</sub> units are perpendicular to each other (torsion angle Cl-B-B-Cl 90°). The B-B distance is 1.70(4) Å, the B-Cl distance is 1.750(5) Å, the Cl-B-Cl angle is 118.7(3)°. B<sub>2</sub>Cl<sub>4</sub> thus differs significantly from B<sub>2</sub>F<sub>4</sub>, which is a planar molecule overall.

Reactions

The compound is used as a reagent for the synthesis of organoboron compounds. For instance, diboron tetrachloride adds to ethylene:

CH<sub>2</sub>=CH<sub>2</sub> + B<sub>2</sub>Cl<sub>4</sub> → Cl<sub>2</sub>B–CH<sub>2</sub>–CH<sub>2</sub>–BCl<sub>2</sub>

Diboron tetrachloride absorbs hydrogen quickly at room temperature:

3 B<sub>2</sub>Cl<sub>4</sub> + 3 H<sub>2</sub> → B<sub>2</sub>H<sub>6</sub> + 4 BCl<sub>3</sub>

With boranes, it replaces a hydrogen to form dichloroborane(3) and a polyhedral dichloroborane. Heat induces disproportionation back to boron trichloride and a polyhedral boron(I) chloride.

References