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Boron sulfide

Boron sulfide is the chemical compound with the formula B<sub>2</sub>S<sub>3</sub>. It is a white, moisture-sensitive solid. It has a polymeric structure. The material has been of interest as a component of "high-tech" glasses and as a reagent for preparing organosulfur compounds. It is the parent member of the thioborates.

Reactions

Like the sulfides of silicon and phosphorus, B<sub>2</sub>S<sub>3</sub> reacts with traces of water, including atmospheric moisture to release H<sub>2</sub>S. This hydrolysis is described by the following idealized equation:

B<sub>2</sub>S<sub>3</sub> readily forms glasses when blended with other sulfides such as P<sub>4</sub>S<sub>10</sub>. Such glasses do not absorb mid-frequencies of Infra-red energy relative to conventional borosilicate glasses. Some of these ternary phases that are fast ion conductors.

B<sub>2</sub>S<sub>3</sub> converts ketones into the corresponding thiones. For example, the conversion of benzophenone to its thione proceeds as follows:

In practice, B<sub>2</sub>S<sub>3</sub> would be used in excess.

Synthesis

An early synthesis involved the reaction of iron and manganese borides with hydrogen sulfide at temperatures of 300&nbsp;°C. The conversion is shown for the monoborides in the following idealized equation:

The first synthesis was done by Jöns Jakob Berzelius in 1824 by direct reaction of amorphous boron with sulfur vapor.

2 B + 3 S → B<sub>2</sub>S<sub>3</sub>

Another synthesis was favoured by Friedrich Wöhler and Henri Etienne Sainte-Claire Deville first published in 1858, starting from boron and hydrogen sulfide.

2 B + 3 H<sub>2</sub>S → B<sub>2</sub>S<sub>3</sub> + 3 H<sub>2</sub>

Structure

The boron atoms in B<sub>2</sub>S<sub>3</sub> are trigonal planar, and are arranged in B<sub>3</sub>S<sub>3</sub> and B<sub>2</sub>S<sub>2</sub> rings with bridging S atoms forming a layer structure with an interlayer distance of 355 pm. This is different from boron trioxide which has a three dimensional structure. The molecular, monomeric, form of B<sub>2</sub>S<sub>3</sub> has a planar V shape with the central B-S-B angle of approximately 120°.

References