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Bis(pinacolato)diboron

Bis(pinacolato)diboron is a covalent compound containing two boron atoms and two pinacolato ligands. It has the formula [(CH<sub>3</sub>)<sub>4</sub>C<sub>2</sub>O<sub>2</sub>B]<sub>2</sub>; the pinacol groups are sometimes abbreviated as "pin", so the structure is sometimes represented as B<sub>2</sub>pin<sub>2</sub>. It is a colourless solid that is soluble in organic solvents. It is a commercially available reagent for making pinacol boronic esters for organic synthesis. Unlike some other diboron compounds, B<sub>2</sub>pin<sub>2</sub> is not moisture-sensitive and can be handled in air.

Preparation and structure

This compound may be prepared by treating tetrakis(dimethylamino)diboron with pinacol in acidic conditions. The B-B bond length is 1.711(6) Å.

Dehydrogenation of pinacolborane provides an alternative route:

2(CH<sub>3</sub>)<sub>4</sub>C<sub>2</sub>O<sub>2</sub>BH → (CH<sub>3</sub>)<sub>4</sub>C<sub>2</sub>O<sub>2</sub>B-BO<sub>2</sub>C<sub>2</sub>(CH<sub>3</sub>)<sub>4</sub> + H<sub>2</sub>

Reactions

The B-B bond adds across alkenes and alkynes to give the 1,2-diborylated alkanes and alkenes. Using various organorhodium or organoiridium catalysts, it can also be installed onto saturated hydrocarbons:

CH<sub>3</sub>(CH<sub>2</sub>)<sub>6</sub>CH<sub>3</sub> + [pinB]<sub>2</sub> → pinBH + CH<sub>3</sub>(CH<sub>2</sub>)<sub>7</sub>Bpin

These reactions proceed via boryl complexes. Bis(pinacolato)diboron can also be used as reducing agent for example in transition metal catalyzed hydrogenations of alkenes and alkynes.

References