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Carbon tetraiodide

Carbon tetraiodide is a tetrahalomethane with the molecular formula . Being bright red, it is a relatively rare example of a highly colored methane derivative. It is only 2.3% by weight carbon, although other methane derivatives are known with still less carbon.

Structure

The tetrahedral molecule features C–I distances of 2.12 ± 0.02 Å. The molecule is slightly crowded with short contacts between iodine atoms of 3.459 ± 0.03 Å, and possibly for this reason, it is thermally and photochemically unstable.

Carbon tetraiodide crystallizes in tetragonal crystal structure (a 6.409, c 9.558 (.10<sup>−1</sup> nm)).

It has zero dipole moment due to its symmetrically substituted tetrahedral geometry.

Properties, synthesis, and uses

Carbon tetraiodide is slightly reactive towards water, giving iodoform and I<sub>2</sub>. It is soluble in nonpolar organic solvents. It decomposes thermally and photochemically to , C<sub>2</sub>I<sub>4</sub>. Its synthesis entails AlCl<sub>3</sub>-catalyzed halide exchange, which is conducted at room temperature:

The product crystallizes from the reaction solution.

Carbon tetraiodide is used as an iodination reagent, often upon reaction with bases. Ketones are converted to 1,1-diiodoalkenes upon treatment with triphenylphosphine (PPh<sub>3</sub>) and carbon tetraiodide. Alcohols are converted in and to iodide, by a mechanism similar to the Appel reaction. In an Appel reaction, carbon tetrachloride is used to generate alkyl chlorides from alcohols.

Safety considerations

Manufacturers recommend that carbon tetraiodide be stored near . As a ready source of iodine, it is an irritant. Its LD<sub>50</sub> on rats is 18&nbsp;mg/kg. In general, organic compounds should be considered toxic, with the narrow exception of small perfluoroalkanes (essentially inert due to the strength of the C–F bond).

References

Further reading