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Samarium(III) sulfide

Samarium(III) sulfide (Sm<sub>2</sub>S<sub>3</sub>) is a chemical compound of the rare earth element samarium, and sulfur. In this compound samarium is in the +3 oxidation state, and sulfur is an anion in the −2 state.

Synthesis

Samarium(III) sulfide can be produced by treating metallic samarium with sulfur:

Once prepared, samarium(III) sulfide can be purified by chemical vapor transport using iodine.

Samarium(III) sulfide can also be prepared by treating the sulfate with hydrogen sulfide at elevated temperatures:

Properties

The low temperature α form crystallises in the orthorhombic crystal system. The unit cell has dimensions a=7.376, b=3.9622 c=15.352&nbsp;Å with volume 448.7&nbsp;Å<sub>3</sub>. There are four of the formula in each unit cell (Sm<sub>8</sub>S<sub>12</sub>). The density comes out to 5.88&nbsp;kg/liter. There are two kinds of samarium coordination in the solid, one is eight coordinated with sulfur surrounding in a bicapped trigonal pyramid. The other is a sevenfold capped distorted octahedral arrangement. This structure is similar to other light rare-earth element sulfides.

Samarium(III) sulfide is a semiconductor with a band gap of 1.7&nbsp;eV. As a thin film on high area electrodes, it is under investigation as a super capacitor dielectric, with specific capacitances of up to 360 Farads per gram.

Related

Related samarium sulfides include the monosulfide SmS and the mixed valent Sm<sub>3</sub>S<sub>4</sub> which are also semiconductors. KSm<sub>2</sub>CuS<sub>6</sub> is a layered quaternary sulfide.

References