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Rhodium(III) iodide

Rhodium(III) iodide is an inorganic compound with the formula RhI<sub>3</sub>. It is a black solid. Some rhodium(III) iodides are used as commercial catalysts.

Structure

RhI<sub>3</sub> adopts same crystal structure motif as AlCl<sub>3</sub> and YCl<sub>3</sub>. The structure consists of cubic close-packed iodide ions and rhodium ions filling a third of the octahedral interstices, forming a layers.

Preparation

Rhodium(III) iodide can be synthesised by the reaction of aqueous potassium iodide with rhodium(III) bromide.

RhBr<sub>3</sub> + 3KI → RhI<sub>3</sub> + 3KBr

Reactivity

Rhodium(III) iodide is only known in the anhydrous form. Unlike the other rhodium(III) halides, it does not form hydrates. The related anion [RhI<sub>6</sub>]<sup>3−</sup> was previously thought not to form but has since been prepared by diffusion of RhCl<sub>3</sub>·3H<sub>2</sub>O through a layer of hydroiodic acid into piperazine.

Although RhI<sub>3</sub> and [RhI<sub>6</sub>]<sup>3−</sup> remain laboratory curiosities, other rhodium(III) iodides have had a major impact technologically. They are catalysts used in the Monsanto process, which at one time was the dominant method for producing acetic acid, a commodity chemical. One intermediate in that cycle is [(CH<sub>3</sub>)Rh(CO)<sub>2</sub>I<sub>3</sub>]<sup>−</sup>.

References