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Niobium oxychloride

Niobium oxychloride is the inorganic compound with the formula NbOCl<sub>3</sub>. It is a white, crystalline, diamagnetic solid. It is often found as an impurity in samples of niobium pentachloride, a common reagent in niobium chemistry.

Structure

In the solid state the coordination sphere for niobium is a distorted octahedron. The Nb–O bonds and Nb–Cl bonds are unequal. This structure can be described as planar Nb<sub>2</sub>Cl<sub>6</sub> core connected by O–Nb–O bridges. In this way, the compound is best described as a polymer, consisting of a double stranded chain.

In the gas phase above 320&nbsp;°C the Raman spectrum is consistent with a pyramidal monomer containing a niobium–oxygen double bond.

Synthesis

Niobium oxychloride is prepared by treating the pentachloride with oxygen:

NbCl<sub>5</sub> + &nbsp;O<sub>2</sub> → NbOCl<sub>3</sub> + Cl<sub>2</sub>

This reaction is conducted at about 200&nbsp;°C. NbOCl<sub>3</sub> also forms as a major side-product in the reaction of niobium pentoxide with various chlorinating agents such as carbon tetrachloride and thionyl chloride.

2&nbsp;Nb<sub>2</sub>O<sub>5</sub> + 6&nbsp;CCl<sub>4</sub> → 4&nbsp;NbOCl<sub>3</sub> + 6&nbsp;COCl<sub>2</sub>

References