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Molybdenum dichloride dioxide

Molybdenum dichloride dioxide is the inorganic compound with the formula . It is a yellow diamagnetic solid that is used as a precursor to other molybdenum compounds. Molybdenum dichloride dioxide is one of several oxychlorides of molybdenum.

Structure

Gaseous molybdenum dichloride dioxide is a monomer, but upon condensation, it polymerizes to give a coordination polymer of uncertain structure.

Preparation

MoO<sub>2</sub>Cl<sub>2</sub> can also be prepared from MoOCl<sub>4</sub>:

MoOCl<sub>4</sub> + O(Si(CH<sub>3</sub>)<sub>3</sub>)<sub>2</sub> → MoO<sub>2</sub>Cl<sub>2</sub> + 2 ClSi(CH<sub>3</sub>)<sub>3</sub>

It is also prepared by chlorination of molybdenum dioxide and molybdenum trioxide:

MoO<sub>2</sub> + Cl<sub>2</sub> → MoO<sub>2</sub>Cl<sub>2</sub>
MoO<sub>3</sub> + Cl<sub>2</sub> → MoO<sub>2</sub>Cl<sub>2</sub>

Reactions

Many bisadducts are known of the type . These octahedral molecular complexes are soluble in organic solvents. The adduct with dimethylsulfoxide can be readily prepared by treatment molybdenum trioxide with concentrated hydrochloric acid:

MoO<sub>3</sub> + 2 HCl + 2 L → MoO<sub>2</sub>Cl<sub>2</sub>L<sub>2</sub> + H<sub>2</sub>O

When treated with bulky anilines, converts to diimido complexes, one of which is . This complex is the precursor to the Schrock carbenes of the type .

References