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Hafnium carbide

Hafnium carbide () is a chemical compound of hafnium and carbon. Previously the material was estimated to have a melting point of about 3,900 Ã‚°C. More recent tests have been able to conclusively prove that the substance has an even higher melting point of 3,958 Ã‚°C exceeding those of tantalum carbide and tantalum hafnium carbide which were both previously estimated to be higher. However, it has a low oxidation resistance, with the oxidation starting at temperatures as low as 430 Ã‚°C. Experimental testing in 2018 confirmed the higher melting point yielding a result of 3,982 (±30°C) with a small possibility that the melting point may even exceed 4,000°C.

Atomistic simulations conducted in 2015 predicted that a similar compound, hafnium carbonitride (HfCN), could have a melting point exceeding even that of hafnium carbide. Experimental evidence gathered in 2020 confirmed that it did indeed have a higher melting point exceeding 4,000 Ã‚°C, with more recent ab initio molecular dynamics calculations predicting the phase to have a melting point as high as 4,110 ± 62 Ã‚°C, highest known for any material.

Hafnium carbide is usually carbon deficient and therefore its composition is often expressed as (x = 0.5 to 1.0). It has a (rock-salt) face-centered cubic crystal structure at any value of x.

Hafnium carbide powder is obtained by the reduction of hafnium(IV) oxide with carbon at 1,800 to 2,000 Ã‚°C. A long processing time is required to remove all oxygen. Alternatively, high-purity HfC coatings can be obtained by chemical vapor deposition from a gas mixture of methane, hydrogen, and vaporized hafnium(IV) chloride.

Because of the technical complexity and high cost of the synthesis, HfC has a very limited use, despite its favorable properties such as high hardness (greater than 9 Mohs) and melting point.

The magnetic properties of change from paramagnetic for x ≤ 0.8 to diamagnetic at larger x. An inverse behavior (dia-paramagnetic transition with increasing x) is observed for , despite its having the same crystal structure as .

See also

References