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Fluorosulfite

Fluorosulfite is an ion with the formula SO<sub>2</sub>F<sup>−</sup>. The term is also used for compounds or salts containing this group. Fluorosulfite was discovered in 1953 by F Seel and H Meier.

Organic compounds with the name "fluorosulfite" contain the group -OS(O)F.

Preparation

[((CH<sub>3</sub>)<sub>2</sub>N)<sub>3</sub>SO][SO<sub>2</sub>F] can be prepared from OSF<sub>4</sub> and Me<sub>3</sub>SiNMe<sub>2</sub>. Alkali metal fluorosulfites can be made by soaking the metal fluoride in liquid sulfur dioxide for a few days. β-CsSO<sub>2</sub>F converts to α-CsSO<sub>2</sub>F when heated to 110&nbsp;°C for a couple of days but remains stable below 50&nbsp;°C.

Properties

The fluorosulfite ion is tetrahedral, with sulfur at the top. The oxygen to sulfur bonds are 147.8&nbsp;pm and the fluorine to sulfur bond is >169.0 pm long. In solid ionic fluorosulfites, the ion is not fixed in orientation and continuously turns around resulting in dynamic disorder. At room temperature this turning rate is from 2×10<sup>5</sup> to 10<sup>7</sup>&nbsp;Hz. When cooled the rate of rotation slows, and can be frozen in place, resulting in static disorder.

Fluorosulfite is isoelectronic with chloryl fluoride (ClO<sub>2</sub>F) and in compounds it resembles chlorate (ClO<sub>3</sub><sup>−</sup>).

The heat of formation from fluoride (F<sup>−</sup>) and sulfur dioxide (SO<sub>2</sub>) is 50 kcal mol<sup>−1</sup>.

Reactions

Fluorosulfites can react with chlorophosphazenes to make fluorophosphazenes:

(NPCl<sub>2</sub>)<sub>n</sub> + 2n KSO<sub>2</sub>F <big>→</big> (NPF<sub>2</sub>)<sub>n</sub> + 2n KCl + 2nSO<sub>2</sub> n=3 or 4

Related

Fluorosulfite is in the category of halosulfite ions which include chlorosulfite, bromosulfite and iodosulfite. Related ions include cyanosulfite SO<sub>2</sub>CN<sup>−</sup>.

List

References