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Europium(III) oxalate

Europium(III) oxalate (Eu<sub>2</sub>(C<sub>2</sub>O<sub>4</sub>)<sub>3</sub>) is a chemical compound of europium and oxalic acid. There are different hydrates including the decahydrate, hexahydrate and tetrahydrate. Europium(II) oxalate is also known.

Preparation

An excess of oxalate is added to a hot solution of Eu<sup>3+</sup> cations. The resulting precipitate of Eu<sub>2</sub>(C<sub>2</sub>O<sub>4</sub>)<sub>3</sub>&nbsp;⋅&nbsp;10H<sub>2</sub>O is dried in a desiccator.

Properties

Europium(III) oxide (Eu<sub>2</sub>O<sub>3</sub>) can be prepared by calcining europium(III) oxalate.

The dehydration of Eu<sub>2</sub>(C<sub>2</sub>O<sub>4</sub>)<sub>3</sub>&nbsp;·&nbsp;10H<sub>2</sub>O occurs below 200&nbsp;°C:

The decomposition of this compound takes place in two stages, the first at 350&nbsp;°C and the second at about 620&nbsp;°C.

In the Mössbauer spectrum, Eu<sub>2</sub>(C<sub>2</sub>O<sub>4</sub>)<sub>3</sub>&nbsp;·&nbsp;10H<sub>2</sub>O shows an isomer shift of +0,26&nbsp;mm/s with a line width of 2,38&nbsp;mm/s, in reference to EuF<sub>3</sub>. The Debye temperature of Eu<sub>2</sub>(C<sub>2</sub>O<sub>4</sub>)<sub>3</sub> is 166±15&nbsp;K.

Eu<sub>2</sub>(C<sub>2</sub>O<sub>4</sub>)<sub>3</sub>&nbsp;·&nbsp;10H<sub>2</sub>O crystallizes monoclinically in the space group of P21/c (space group no. 14) with the lattice parameters a = 1098, b = 961, c = 1004 pm and β = 114.2° with four formula units per unit cell.

Nanoparticles show a line emission when excited by a light source of 393&nbsp;nm, the transitions <sup>5</sup>D<sub>0</sub>→<sup>7</sup>F<sub>1</sub> (592&nbsp;nm) and <sup>5</sup>D<sub>0</sub>→<sup>7</sup>F<sub>2</sub> (616&nbsp;nm) can then be found in the spectrum. This can be used as a red phosphor for white LEDs.

References