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Ethenedithione

Ethenedithione or ethylenedithone is an unstable chemical substance with formula S=C=C=S made from carbon and sulfur.

Ethenedithione can exist as a gas at low pressure and high temperature, but is unstable when condensed or under higher pressure.

It can be stabilized as a ligand binding two cobalt atoms.

Other occurrences as a ligand are in TpW(CO)<sub>2</sub>(C<sub>2</sub>S<sub>2</sub>)<sup>–</sup> and [TpW(CO)<sub>2</sub>]<sub>2</sub>Ni(C<sub>2</sub>S<sub>2</sub>)<sub>2</sub>, where Tp is trispyrazolylborate.

Formation

Ethenedithione can be made by the flash vacuum pyrolysis of 2,5-Dithiacyclopentylideneketene.

Also it has been made by dissociative ionization of tetrathiapentalenedione, and then neutralisation of ions produced.

C<sub>2</sub>S<sub>2</sub> is made along with carbon subsulfide and carbon monosulfide, in an electric discharge in carbon disulfide vapour.

Properties

In its ground state it is a triplet state (<sup>3</sup>Σ<sub>g</sub><sup>−</sup>). Ethenedithione can be trapped in a matrix of solid argon without decomposition.

The infrared spectrum contains a prominent line at 1179.3&nbsp;cm<sup>−1</sup> due to asymmetric C=S stretch of the most common isotopes.

Over 60 K, ethenedithione polymerises. Possible polymerisation products include polythiene.

References