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Dysprosium(III) carbonate

Dysprosium(III) carbonate is an inorganic compound with the chemical formula Dy<sub>2</sub>(CO<sub>3</sub>)<sub>3</sub>. It is a white, paramagnetic solid.

Properties

An amorphous tetrahydrate exists, stable in air up to near the decomposition temperature. It progressively looses water upon heating and is directly converted to dysprosium oxide (Dy<sub>2</sub>O<sub>3</sub>) by dehydration and carbonate calcination:

Dy<sub>2</sub>(CO<sub>3</sub>)<sub>3</sub>·xH<sub>2</sub>O → Dy<sub>2</sub>O<sub>3</sub> + xH<sub>2</sub>O + 3 CO<sub>2</sub>

An orthorhombic kozoite-type DyCO<sub>3</sub>OH forms under hydrothermal conditions, and a poorly crystalline tengerite-type Dy<sub>2</sub>(CO<sub>3</sub>)·2-3H<sub>2</sub>O remains stable at ambient temperature.

Preparation

Dysprosium(III) carbonate can be prepared by reacting a soluble dysprosium salt such as dysprosium(III) chloride with sodium carbonate, forming a white gel-like precipitate. The flow rate of the Dy(III) solution and the reactor temperature affect the particle size of the product.

Another method involves the hydrolysis of dysprosium trichloroacetate in a homogeneous phase reaction:

2 Dy(Cl<sub>3</sub>CCOO)<sub>3</sub> + (x+3)H<sub>2</sub>O → Dy<sub>2</sub>(CO<sub>3</sub>)<sub>3</sub>·xH<sub>2</sub>O + 3 CO<sub>2</sub> + 6 CHCl<sub>3</sub>

Carbon dioxide and chloroform are formed as byproducts in this reaction.

It can also be prepared by passing carbon dioxide through a suspension of dysprosium hydroxide or oxide in water. The conversion is slow and may not produce a pure product. The reaction is fast with higher yields if supercritical CO<sub>2</sub> at high pressure is used instead.

Uses

It can be used as a photocatalyst for the degradation of methyl orange under ultraviolet light.

Related compounds

The crystal structures of the hydroxide carbonate (DyOHCO<sub>3</sub>) and another basic carbonate (Dy<sub>2</sub>O<sub>2</sub>CO<sub>3</sub>) have been determined. They can be prepared by hydrothermal synthesis involving the reaction of dysprosium(III) chloride and carbon dioxide with caesium carbonate and potassium carbonate respectively.

The dysprosium tetracarbonate complex [C(NH<sub>2</sub>)<sub>3</sub>]<sub>4</sub>[Dy(CO<sub>3</sub>)<sub>4</sub>(H<sub>2</sub>O)](H<sub>3</sub>O)·13H<sub>2</sub>O has been characterized by single-crystal X-ray diffraction. It can be prepared by treating saturated guanidinium carbonate solution with dysprosium nitrate.

References