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Cyclopentadienyl allyl palladium

Cyclopentadienyl allyl palladium is an organopalladium compound with formula (C<sub>5</sub>H<sub>5</sub>)Pd(C<sub>3</sub>H<sub>5</sub>). This reddish solid is volatile with an unpleasant odor. It is soluble in common organic solvents. The molecule consists of a Pd centre sandwiched between a Cp and allyl ligands.

Preparation

This complex is produced by the reaction of allylpalladium chloride dimer with sodium cyclopentadienide:

2 C<sub>5</sub>H<sub>5</sub>Na + (C<sub>3</sub>H<sub>5</sub>)<sub>2</sub>Pd<sub>2</sub>Cl<sub>2</sub> → 2 (C<sub>5</sub>H<sub>4</sub>)Pd(C<sub>3</sub>H<sub>5</sub>) + 2 NaCl

Structure and reactions

The 18-electron complex adopts a half-sandwich structure with C<sub>s</sub> symmetry, i.e., the molecule has a plane of symmetry. The complex can be decomposed readily by reductive elimination.

C<sub>3</sub>H<sub>5</sub>PdC<sub>3</sub>H<sub>5</sub> → Pd(0) + C<sub>5</sub>H<sub>5</sub>C<sub>3</sub>H<sub>5</sub>

The compound readily reacts with alkyl isocyanides to produce clusters with the approximate formula [Pd(CNR)<sub>2</sub>]<sub>n</sub>. It reacts with bulky alkyl phosphines to produce two-coordinated palladium(0) complexes:

CpPd(allyl) + 2 PR<sub>3</sub> → Pd(PR<sub>3</sub>)<sub>2</sub> + C<sub>5</sub>H<sub>5</sub>C<sub>3</sub>H<sub>5</sub>

The compound has been used to deposit thin film chemical vapor deposition of metallic palladium.

References