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Cerocene

Cerocene is a organometallic complex with the chemical formula Ce(C<sub>8</sub>H<sub>8</sub>)<sub>2</sub> (Ce(cot)<sub>2</sub>). It is a sandwich compound consisting of a central cerium atom and two cyclooctatetraenide rings.

Preparation

Cerocene can be prepared by reducing cerium(III) di-cyclooctatraene anion salts:

Ce(C<sub>8</sub>H<sub>8</sub>)<sub>2</sub>K → Ce(C<sub>8</sub>H<sub>8</sub>)<sub>2</sub> + K<sup>+</sup>

Chemical properties

Cerocene decomposes when exposed to water or oxygen to yield non-stoichiometric cerium-oxides and cyclooctratraene derivitives.

It undergoes a disproportionation, leading to an equilibrium between cerocene and a double-decker structure containing two cerium atoms:

2 Ce(C<sub>8</sub>H<sub>8</sub>)<sub>2</sub> Ce<sub>2</sub>(C<sub>8</sub>H<sub>8</sub>)<sub>3</sub> + C<sub>8</sub>H<sub>8</sub>

Although the cyclooctatetraenide ligand is usually considered a dianion and therefore cerocene is identified as a Ce(IV) complex, theoretical and experimental analysis of the compound indicates that is more correctly described containing a Ce(III) atom.

Related compounds

Cerocene is a known precursor for uranocene, U(C<sub>8</sub>H<sub>8</sub>)<sub>2</sub>:

Ce(C<sub>8</sub>H<sub>8</sub>)<sub>2</sub> + UCl<sub>3</sub> U(C<sub>8</sub>H<sub>8</sub>)<sub>2</sub> + CeCl<sub>3</sub>

Cerocene is commonly confused with the compound tris(cyclopentadienyl)cerium.

References